The degree set of a graph is the set of degrees of its vertices. It has been shown that when the cardinality of is (i.e., is regular) or (i.e., is bi-regular), the balance index set of has simple structures. In this work, we determine the balance index sets of unicyclic graphs and subclasses of graphs to demonstrate the application of this recent result. In addition, we give an explicit formula for the balance index sets of subclasses of complete tri-bipartite graphs (). Structural properties regarding the balance index sets of a general graph and application examples are also presented.